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天然气 11

普光气田 7

勘探开发 6

页岩气 5

天然气水合物 4

温室气体 4

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WO₃ nanomaterials synthesized via a sol-gel method and calcination for use as a CO gas sensor

Diah SUSANTI,A.A. Gede Pradnyana DIPUTRA,Lucky TANANTA,Hariyati PURWANINGSIH,George Endri KUSUMA,Chenhao WANG,Shaoju SHIH,Yingsheng HUANG

《化学科学与工程前沿（英文）》 2014年第8卷第2期页码 179-187 doi: 10.1007/s11705-014-1431-0

摘要： Carbon monoxide is a poisonous and hazardous gas and sensitive sensor devices are needed to prevent humans from being poisoned by this gas. A CO gas sensor has been prepared from WO synthesized by a sol-gel method. The sensor chip was prepared by a spin-coating technique which deposited a thin film of WO on an alumina substrate. The chip samples were then calcined at 300, 400, 500 or 600 °C for 1 h. The sensitivities of the different sensor chips for CO gas were determined by comparing the changes in electrical resistance in the absence and presence of 50 ppm of CO gas at 200 °C. The WO calcined at 500 °C had the highest sensitivity. The sensitivity of this sensor was also measured at CO concentrations of 100 ppm and 200 ppm and at operating temperatures of 30 and 100 °C. Thermogravimetric analysis of the WO calcined at 500 °C indicated that this sample had the highest gas adsorption capacity. This preliminary research has shown that WO can serve as a CO gas sensor and that is should be further explored and developed.

关键词： WO₃ nanomaterial sol-gel calcinations CO gas sensor sensitivity

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CO, N, and CO/N mixed gas injection for enhanced shale gas recovery and CO geological storage

《能源前沿（英文）》 2023年第17卷第3期页码 428-445 doi: 10.1007/s11708-023-0865-9

摘要： In this work, using fractured shale cores, isothermal adsorption experiments and core flooding tests were conducted to investigate the performance of injecting different gases to enhance shale gas recovery and CO₂ geological storage efficiency under real reservoir conditions. The adsorption process of shale to different gases was in agreement with the extended-Langmuir model, and the adsorption capacity of CO₂ was the largest, followed by CH_4, and that of N₂ was the smallest of the three pure gases. In addition, when the CO₂ concentration in the mixed gas exceeded 50%, the adsorption capacity of the mixed gas was greater than that of CH₄, and had a strong competitive adsorption effect. For the core flooding tests, pure gas injection showed that the breakthrough time of CO₂ was longer than that of N₂, and the CH₄ recovery factor at the breakthrough time (

R C H 4

) was also higher than that of N₂. The

R C H 4

of CO₂ gas injection was approximately 44.09%, while the

R C H 4

of N₂ was only 31.63%. For CO₂/N₂ mixed gas injection, with the increase of CO₂ concentration, the

R C H 4

increased, and the

R C H 4

for mixed gas CO₂/N₂ = 8:2 was close to that of pure CO₂, about 40.24%. Moreover, the breakthrough time of N₂ in mixed gas was not much different from that when pure N₂ was injected, while the breakthrough time of CO₂ was prolonged, which indicated that with the increase of N₂ concentration in the mixed gas, the breakthrough time of CO₂ could be extended. Furthermore, an abnormal surge of N₂ concentration in the produced gas was observed after N₂ breakthrough. In regards to CO₂ storage efficiency (

S s t o r a g e - C O 2

), as the CO₂ concentration increased,

S s t o r a g e - C O 2

also increased. The

S s t o r a g e - C O 2

of the pure CO₂ gas injection was about 35.96%, while for mixed gas CO₂/N₂ = 8:2,

S s t o r a g e - C O 2

was about 32.28%.

关键词： shale gas gas injection competitive adsorption enhanced shale gas recovery CO₂ geological storage

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自然对流气体的摆特性及其在传感器中应用

张福学

《中国工程科学》 2002年第4卷第8期页码 50-53

摘要：

根据自然对流气体具有摆的特性，从而提出气体摆新概念。分析了密闭腔中自然对流气体的浮升力，给出浮升力与温度变化的关系式。试验结果表明，与固体摆、液体摆一样，利用气体摆原理亦能检测加速度和倾角。

关键词：气体的摆特性倾角传感器加速度计

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Catalytic performance of Co-Mo-Ce-K/γ-Al

Yuqiong ZHAO, Yongfa ZHANG

《化学科学与工程前沿（英文）》 2010年第4卷第4期页码 457-460 doi: 10.1007/s11705-010-0524-7

摘要： The catalytic performance of Co-Mo-Ce-K/γ-Al O catalyst for the shift reaction of CO in coke oven gas is investigated using X-ray diffraction (XRD) and temperature-programmed reduction (TPR). The results indicate that Ce and K have a synergistic effect on promoting the catalytic activity, and the Co-Mo-Ce-K/γ-Al O catalyst with 3.0 wt-% CeO and 6.0 wt-% K O exhibits the highest activity. CeO favors Co dispersion and mainly produces an electronic effect. TPR characterization results indicate that the addition of CeO -K O in the Co-Mo-Ce-K/γ-Al O catalyst decreases the reduction temperature of active components, and part of octahedrally coordinated Mo transforms into tetrahedrally coordinated Mo , which has a close relationship with the catalytic activity.

关键词： coke oven gas water gas shift reaction sulfur-tolerant catalyst cerium dioxide

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Greenhouse gas emissions during co-composting of cattle feedlot manure with construction and demolition

Xiying Hao, Francis J. Larney

《环境科学与工程前沿（英文）》 2017年第11卷第3期 doi: 10.1007/s11783-017-0955-1

摘要： Manure management strategies should reflect current animal feeding practices and encourage recycling of organic waste to help protect our environment. This research investigated greenhouse gas (GHG) emissions during cattle manure stockpiling or composting with and without construction and demolition (C&D) waste. Manure was collected from cattle fed a typical finishing diet (CK manure) and from cattle on diets which included 30% dried distillers grains with solubles (DG manure). The CK and DG manures were co-composted with (4:1) C&D waste (treatments: CK_CD DG_CD), composted alone (treatments: CK and DG) in 13 m bins or stockpiled without C&D waste (treatments: CK_ST and DG_ST) for 99 days. Manure type (CK vs. DG manure) had no effect on GHG emissions over the 99 day manure composting or stockpiling. Composting with C&D waste produced similar CO emissions, about double that from manure stockpiling (7.0 kgC·m ). In contrast, CH emissions were reduced by the inclusion of C&D waste (64 gC·m with C&D vs. 244 gC·m without C&D) while the manure stockpile emitted the greatest amount of CH (464 gC·m ). Additionally, only 0.48% of C was emitted in CH form with C&D waste, compared to 1.68% when composting without C&D waste and 7.00% when cattle manure was stockpiled. The N O emissions (12.4 to 18.0 gN·m ) were similar across all treatments. The lower CH emissions with C&D waste are beneficial in reducing overall GHG emissions from manure composting, while reducing the amount of material entering landfills.

关键词： Livestock manure greenhouse gas flux straw bale compost bin N₂O CH₄ CO₂

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Lagrangian simulation of deposition of CO gas-solid sudden expansion flow

HUANG Dongping, DING Guoliang, QUACK Hans

《能源前沿（英文）》 2008年第2卷第2期页码 216-221 doi: 10.1007/s11708-008-0032-3

摘要： Freezing and blockage resulting from the deposition of solid CO formed because of sudden expansion of the downstream pipe during the release of CO through safety valves, will endanger the protected equipment. To overcome this problem, the characteristics of the CO gas-solid sudden expansion flow are studied by using the disperse Lagrangian model. A comparison of the calculated deposition of the solid CO with the experimental results shows that they are in reasonable agreement. The simulation results show that the size of the solid CO formed should not be in the range of 0.04–0.07 mm ( number 3.2–9.8). This can be achieved by using an appropriate flow cross section of the safety valve.

关键词： comparison gas-solid downstream blockage Lagrangian

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页岩气网络设计与运行之间的相互作用，包括CO₂固存

Sharifzadeh Mahdi, Xingzhi Wang, Nilay Shah

《工程（英文）》 2017年第3卷第2期页码 244-256 doi: 10.1016/J.ENG.2017.02.007

摘要：但是，由于页岩气储层的渗透率极低，因此可能需要按顺序进行特殊程序，例如水平钻井，水力压裂，定期关井和注入二氧化碳（CO ₂）以提高天然气产量，最大程度地提高经济效益，并确保安全和无害环境的运营接下来，我们对重要设计和操作决策进行敏感性分析，例如井长，井眼布置，裂缝数量，裂缝距离，CO ₂注入速率和闭井调度，以获取增产效果。对页岩气网络复杂行为的深入见解。钻探，压裂和CO ₂注入对这项技术的经济可行性具有重大影响。尤其是，由于成本高昂，除非使用CO ₂减税或补贴，否则使用CO ₂的增强气体回收（EGR）似乎不具有商业竞争力。隔离。

关键词：页岩气，水力压裂，调度，完井，CO ₂隔离，同时优化

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Review on cryogenic technologies for CO removal from natural gas

Yujing BI, Yonglin JU

《能源前沿（英文）》 2022年第16卷第5期页码 793-811 doi: 10.1007/s11708-022-0821-0

摘要： CO₂ in natural gas (NG) is prone to condense directly from gas to solid or solidify from liquid to solid at low temperatures due to its high triple point and boiling temperature, which can cause a block of equipment. Meanwhile, CO₂ will also affect the calorific value of NG. Based on the above reasons, CO₂ must be removed during the NG liquefaction process. Compared with conventional methods, cryogenic technologies for CO₂ removal from NG have attracted wide attention due to their non-polluting and low-cost advantages. Its integration with NG liquefaction can make rational use of the cold energy and realize the purification of NG and the production of by-product liquid CO₂. In this paper, the phase behavior of the CH₄-CO₂ binary mixture is summarized, which provides a basis for the process design of cryogenic CO₂ removal from NG. Then, the detailed techniques of design and optimization for cryogenic CO₂ removal in recent years are summarized, including the gas-liquid phase change technique and the gas-solid phase change technique. Finally, several improvements for further development of the cryogenic CO₂ removal process are proposed. The removal process in combination with the phase change and the traditional techniques with renewable energy will be the broad prospect for future development.

关键词： cryogenic CO₂ removal purification of natural gas (NG) biogas upgrading CH₄-CO₂ binary system

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Experimental study on capturing CO 2 greenhouse gas by mixture of ammonia and soil

Ying WU, Yifei WANG, Qinghua ZENG, Xin GONG, Zunhong YU,

《化学科学与工程前沿（英文）》 2009年第3卷第4期页码 468-473 doi: 10.1007/s11705-009-0257-7

摘要： This paper presents our study on removal of carbon dioxide (CO) greenhouse gas emissions by using the mixture of ammonia and soil. CO capture capacity using this method is 15% higher than the sum of ammonia chemical absorption capacity and soil physical adsorption capacity. Scanning electron microscopy (SEM) and Fourier transform infrared spectroscopy (FTIR) are utilized to study this synergism. The removal effect is not only reflected in ammonia chemical reaction with CO. CO can also be absorbed by ammonium bicarbonate (NHHCO) crystal, which is the main component of the product, or wrapped in the pore of the crystal or packed in the gap between the crystal and the soil. CO can be permanently deposited as carbonated minerals in the subsoil earth layers.

关键词： electron microscopy product physical adsorption capacity spectroscopy

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Corrigendum to “Interactions between the Design and Operation of Shale Gas Networks, IncludingCO2 Sequestration” [Engineering (2017) 244–256] Corrigendum

Mahdi Sharifzadeh,Xingzhi Wang,Nilay Shah

《工程（英文）》 2017年第3卷第3期页码 429-429 doi: 10.1016/J.ENG.2017.03.027

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温室气体提高采收率的资源化利用及地下埋存

沈平平,江怀友

《中国工程科学》 2009年第11卷第5期页码 54-59

摘要：建立适合中国国情的CO₂高效利用和埋存体系；实现CO₂减排的社会效益和CO₂高效利用的经济效益；发展适合中国国情的CO₂埋存地下理论、多相多组分相态理论、多相多组分非线性渗流理论和CO₂捕集与储运理论。通过上述基础研究，形成具有自主知识产权的CO₂地质埋存和高效利用的综合技术，使中国CO₂安全埋存—高效利用研究处于国际水平。

关键词：温室气体资源化利用 CO2地下埋存提高采收率

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普光气田地面集输系统的内腐蚀控制与监测

欧莉,李时杰,苏国丰

《中国工程科学》 2010年第12卷第10期页码 70-75

摘要：

分析了高含H₂S / CO₂气田的腐蚀特征，探讨了在普光气田开发建设同期模拟普光集输工况开展的腐蚀性研究与成果

关键词：普光酸性气田 H2S CO2 湿气输送缓蚀剂腐蚀监测

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南海富碳天然气直接利用技术发展研究

吴青,于广欣,汤晓玲,张亮亮,郑裕国

《中国工程科学》 2021年第23卷第4期页码 172-181 doi: 10.15302/J-SSCAE-2021.04.020

摘要：

我国南海富碳天然气具有 CO₂ 含量高的特点，高效开发和精准利用南海富碳天然气资源，有助于积极应对气候变化，实现&ldquo本文分析了南海富碳天然气直接利用的需求和价值，概括了富碳天然气直接利用的发展现状；重点论述了富碳天然气 CO₂-CH₄ 干重整技术、富碳天然气制甲醇一体化技术、富碳天然气 CO₂ 加氢制液体燃料技术、富碳天然气直接制精细化工品技术等的实施过程与应用特征。

关键词：南海富碳天然气干重整 CO2 加氢液体燃料精细化工

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凝析气藏的经济开采模式

刘廷元

《中国工程科学》 2001年第3卷第3期页码 85-91

摘要：介绍了国外近20 a来在凝析气藏开采技术领域的各种经济模式，包括回注φ_d=75%干气、自流回注、注N₂、注水、水气交替注和注CO₂

关键词：凝析气藏开采模式注气注氮注水注二氧化碳经济

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油气田监测高性能微传感器及数字化系统

赵玉龙,牛喆,周冠武,赵立波,蒋庄德

《中国工程科学》 2013年第15卷第1期页码 99-105

摘要：

针对油气田特殊环境要求，介绍了一种高温高压传感器芯片的设计及加工制造方法，并研发了相关的高性能数字变送系统。所设计的高温高压传感器芯片解决了传统压阻式传感器在高温高压环境下的热稳定性问题，通过数字补偿技术进一步提升了其系统的线性度与精度，并针对油气田监测环境扩展了其相关外围设备。同时，为了适应油气田管监测理要求，设计了相关无线传感网络，以确保其工业生产的高效运行和有效控制。通过具体实验测试数据，验证了该油气田监测高性能微传感器及数字化系统的高精度及高可靠性，该系统的精度达到0.2 % FS及以上，达到世界先进水平，对国内的石化工业发展有着非常重要的意义。

关键词：高温高压传感器芯片高性能数字变送系统数字补偿技术无线传感网络高精度